I am certainly not an expert on welding Cr-Mo tubing with undermatching filler metal, but I can tell you a few things about the fillers you are questioning about.
First thing, is the R60 you are using is actually an oxy-fuel mild steel welding rod. The tensile strength is 60 ksi or 413 MPa. The ER70S-2 and ER70S-6 have a 70 ksi tensile strength, or 482 MPa. The main difference between them is the ER70S-6 has more deoxidizers (Si and Mn). The specification for these is AWS A5.18. The ER80S-D2 is found in AWS A5.28, and has alloy additions of 1 3/4 Mn and 1/2 Mo. Tensile strenght is 80 ksi or 551 MPa. Minimum elongations for ER80S-D2 is 17% as welded, and for both ER70S-2 & 6 is 22% minimum. These are just the minimum specified though. For actual results, you might check out the ESAB, Hobart, or Lincoln Electric websites. They usually have that info on data sheets.